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Many adsorbate phases are "floating" on the substrate surface, in the sense that the adsorbate-substrate interaction is sufficient to cause commensurability, but insufficient to cause a significant structural change at the surface, such as a reconstruction. 1). g. for H adsorbed on Ni(110) [81Eng, 84Pen]. The subject will be briefly discussed by the example of H adsorbed on Fe(110) [77Boz, 82Imb, 83Sel]. 67, respectively. Less sharp streaky patterns were seen for intermediate coverages. e. superstructure) LEED spots versus temperature in the range 150-300 K, an order-disorder transition was monitored at nearly constant H coverages.
Deduced a mixture of CO bonding to a single (atop) and two adjacent Ni surface atoms (bridge site) at low CO coverage and exclusively to bridge sites at high CO coverage. Voigtländer et al. favored the atop site Landolt-Börnstein New Series III/42A Ref. p. 59] 1 Introduction 29 at high coverage. Structural investigations proved the bridge site to be correct at the high CO coverage of the ordered CO (2×1)p2mg layer [88Han, 93Hua, 93Pan1, 93Pan2]. 003 A resolution = 7 cm 2060 –1 Fig. 22. 57. All peaks correspond to C–O stretch vibrations [88Sur].
An increase in activation energies for both diffusion directions if found at lower CO coverages, as seen by the example (d) [93Xia]. 9 kcal/mol which is higher than on Ni(110). The calculated diffusion coefficients fall into the same range as those of Landolt-Börnstein New Series III/42A 1 Introduction 24 [Ref. p. 59 the lower group in Fig. 15 [88Zhu, 90Lin]. It is interesting to note that two very different techniques, one of them also a local probe of diffusion [90Lin], have produced a fairly consistent set of data for CO/Ni(111).